Thermoplastic Multilayer Composites - ifm kit

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Continuum mechanical modelling of deformation and failure mechanisms in thermoplastic multilayer composites Thomas Seelig Institute of Mechanics, Karlsruhe University, Germany, [email protected]

Introduction (a)

• tensile response of PC/SAN multilayer composites controlled by interacting micromechanisms - shear banding in (ductile) PC

PC

(b) PC

PC

- crazing / microcracking in (brittle) SAN - formation of network-like deformation pattern at small overall strain (a) • macroscopic behaviour: brittle failure of SAN-rich composites (PC content / relative layer thickness < 50%) due to early coalescence of microcracks ductile response of PC-rich composites (> 50 %), holes in SAN grown from microcracks are stabilised (b) (from: Gregory, B.L. et al., J. Mat. Sci. 1987, 22, 532-538)

 objective of present study: gain additional understanding of interrelation between microstructure, micromechanisms and macroscopic behaviour from numerical (finite element) simulations

Modeling Bulk constitutive models:

- sample with alternating layers of PC and SAN, plane strain (2D) model - uniaxial overall loading in terms of prescribed macroscopic strain rate ε&

PC: finite strain viscoplasticity,

- cohesive surfaces as potential locations of failure cohesive failure modes: - crazing in SAN

.

ε SAN

PC

SAN

PC

- ductile rupture of PC upon large plastic deformation

SAN

σ SAN

intrinsic softening ( shear banding),

PC

rehardening due to molecular alignment

(uniaxial tension)

SAN: linear elastic (tension)

ε cohesive surfaces

Cohesive zone model for crazing: - initiation criterion (crit. normal stress)

SAN

PC

- rate-dependent traction-separation law

σc

∆& C (T&,T ;σ C )

∆c T

- craze widening resistance σ C (∆ C ) (micromechanics of fibrillation process) - craze-breakdown at crit. craze width

cr

∆c

Results - simulations with different realisations (statistically equivalent) of initial defect distribution in σ [MPa] SAN (lower craze initiation stress) 70 - composition-dependent overall brittle-to-ductile transition 60 reproduced 50 - localisation of damage in 40 SAN-rich composites (a) and early brittle failure 30 - spatially distributed damage in 20 PC-rich composites (b, c) and 10 ductile overall behaviour 0 - long-range extension of shear band network (scaling with relative PC layer thickness) plays pivotal role for delocalisation of damage

macroscopic response

contours of local plastic strain (c)

PC/SAN (3/1)

(b)

(b)

(a) εp

(c) ε

PC/SAN (1/3)

ε

0.5 0.4 0.3 0.2 0.1 0.0

(a) 0

0.05

p

0.1

0.15

p 0.5 0.4 0.3 0.2 0.1 0.0

ε PC/SAN(1/3)

PC/SAN(3/1)

1.2 1.0 0.8 0.6 0.4 0.2 0.0

∆c